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Anti-corrosive agents based benzil-thiocarbohydrazone macrocyclic ligand-derived Cu (II) and Zn (II) chelates: template synthesis and physically admixing with epoxy coating

Walid E. Elgammal (Department of Chemistry, Faculty of Science, Al-Azhar University, Cairo, Egypt)
Essam M. Eliwa (Department of Chemistry, Faculty of Science, Al-Azhar University, Cairo, Egypt)
Hosni A. Goomaa (Department of Chemistry, Faculty of Science, Al-Azhar University, Cairo, Egypt)
Medhat E. Owda (Department of Chemistry, Faculty of Science, Al-Azhar University, Cairo, Egypt)
H. Abd El-Wahab (Department of Chemistry, Faculty of Science, Al-Azhar University, Cairo, Egypt)

Pigment & Resin Technology

ISSN: 0369-9420

Article publication date: 2 March 2023

Issue publication date: 15 July 2024

103

Abstract

Purpose

This paper aims to focus on the synthesis of the macrocyclic complexes (Cu and Zn) and their applications as anticorrosive materials in epoxy paint formulation for surface coating application.

Design/methodology/approach

A selected macrocyclic Cu(II) and Zn(II) complexes were prepared via template synthesis and characterized using Fourier transform infrared, thermal gravimetric analysis, scanning electron microscope, flexibility, hardness and adhesion of coating films prepared using epoxy paint.

Findings

The corrosion resistance of the epoxy-painted films was improved due to the incorporation of the Zn and Cu complexes into the formulation.

Originality/value

It was found that the metal complex-based formulation with Cu(II) and Zn(II) had outperformed the sample blank.

Keywords

Acknowledgements

Author contributions: All authors contributed equally to this manuscript.

Funding declaration: There is no funding.

Ethical approval: There is no ethical approval due to this study not including human or animal studies.

Conflicts of interest: The authors declare no competing financial.

Data availability statements: Any data related to this manuscript can be made available on request.

Citation

Elgammal, W.E., Eliwa, E.M., Goomaa, H.A., Owda, M.E. and Abd El-Wahab, H. (2024), "Anti-corrosive agents based benzil-thiocarbohydrazone macrocyclic ligand-derived Cu (II) and Zn (II) chelates: template synthesis and physically admixing with epoxy coating", Pigment & Resin Technology, Vol. 53 No. 5, pp. 595-603. https://doi.org/10.1108/PRT-11-2022-0132

Publisher

:

Emerald Publishing Limited

Copyright © 2023, Emerald Publishing Limited

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